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Time-reversal-symmetry breaking and unconventional pairing in the noncentrosymmetric superconductor La7Rh3

D. Singh, M. S. Scheurer, A. D. Hillier, D. T. Adroja, R. P. Singh

DOI 10.1103/PhysRevB.102.134511 · Physical Review B

T1

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Abstract

Noncentrosymmetric superconductors have sparked significant research interests due to their exciting properties, such as the admixture of spin-singlet and spin-triplet pairing. Here we report on the muon spin rotation and relaxation and thermodynamic measurements on the noncentrosymmetric superconductor La7Rh3, which show an isotropic superconducting gap but also spontaneous time-reversal-symmetry breaking occurring at the onset of superconductivity. We show that our results pose severe constraints on any microscopic theory of superconductivity in this system. A symmetry analysis identifies ground states compatible with time-reversal-symmetry breaking, and the resulting gap functions are discussed. Furthermore, general energetic considerations indicate the relevance of electron-electron interactions for the pairing mechanism, in accordance with hints of spin fluctuations revealed in susceptibility measurements.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
La7Rh3

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2.65Pressure not reportedonset
La7Rh3

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2.65Pressure not reportedonset
La7Rh3

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2.64Pressure not reportedonset
Sr2RuO4

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—Pressure not reportedunknown
UPt3

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—Pressure not reportedunknown
PrPt4Ge12

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—Pressure not reportedunknown
LaNiGa2

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—Pressure not reportedunknown
Lu5Rh6Sn18

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—Pressure not reportedunknown
Ba0.27K0.73Fe2As2

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—Pressure not reportedunknown
LaNiC2

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

—Pressure not reportedunknown
Re6Zr

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—Pressure not reportedunknown
Re6Hf

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—Pressure not reportedunknown
SrPtAs

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—Pressure not reportedunknown
La7Ir3

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—Pressure not reportedunknown

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