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Unified theory of spin and charge excitations in high-Tc cuprate superconductors: A quantitative comparison with experiment and interpretation

Maciej Fidrysiak, Józef Spałek

DOI 10.1103/PhysRevB.104.L020510 · Physical Review B

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Abstract

We provide a unified interpretation of both paramagnon and plasmon modes in high-Tc copper-oxides, and verify it quantitatively against available resonant inelastic x-ray scattering (RIXS) data across the hole-doped phase diagram. The three-dimensional extended Hubbard model, with included long-range Coulomb interactions and doping-independent microscopic parameters for both classes of quantum fluctuations, is used. Collective modes are studied using VWF+1/Nf approach which extends variational wave function (VWF) scheme by means of an expansion in inverse number of fermionic flavors (1/Nf). We show that intense paramagnons persist along the antinodal line from the underdoped to the overdoped regime and undergo rapid overdamping in the nodal direction. Plasmons exhibit a three-dimensional character, with minimal energy corresponding to antiphase oscillations on neighboring CuO2 planes. The theoretical spin- and charge excitation energies reproduce semiquantitatively RIXS data for (Bi,Pb)2(Sr,La)2CuO6+δ. The present VWF+1/Nf analysis of dynamics and former VWF results for static quantities combine into a consistent description of the principal properties of hole-doped high-Tc cuprates as strongly correlated systems.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
(Bi,Pb)2(Sr,La)2CuO6+δ

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

—Pressure not reportedunknown
Bi2Sr1.6La0.4CuO6+δ

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

—Pressure not reportedunknown

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