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Pressure effect in the antiperovskite phosphide superconductor Sr(Pt0.9Pd0.1)3P

Lifen Shi, Pengtao Yang, Teng Wang, Pengfei Shan, Ziyi Liu, Shuxiang Xu, Keyu Chen, Ningning Wang, Long Zhou, Youwen Long, Jianping Sun, Gang Mu, Yoshiya Uwatoko, Bosen Wang, Jinguang Cheng

DOI 10.1103/PhysRevB.105.214529 · Physical Review B

T1

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Abstract

We report a high-pressure study on the antiperovskite phosphide superconductor Sr(Pt0.9Pd0.1)3P. The superconducting transition temperature Tc decreases with a negative differential pressure coefficient, dlnTc/dP≈–0.052GPa–1 (dTc/dP≈–0.33K/GPa for P<10GPa), which is a very high value for antiperovskite superconductors. We find that the upper critical field μ0Hc2(0) also decreases with increasing pressure, but the μ0Hc2(0)/kBTc, e.g., 2Δ0[πN(EF)]1/2/kBTc, is doubled from ∼0.5–0.7 T/K at ambient pressure to ∼1.2 T/K at 31.7 GPa. Our comparative studies on the dependences of Tc as functions of physical pressure versus chemical doping support that Sr(Pt0.9Pd0.1)3P belongs to a phonon-mediated Bardeen-Cooper-Schrieffer-type superconductor with enhanced superconducting coupling strengths. The reduction of Tc with pressure should mainly originate from the decrease of the density of states at the Fermi level and the phonon-hardening effect. Our results shed some light on understanding the superconducting mechanisms of Pt-based antiperovskite superconductors.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
Sr(Pt0.9Pd0.1)3P

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8.1Pressure unresolvedonset
Sr(Pt0.9Pd0.1)3P

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7.2Pressure unresolvedzero_resistance
Sr(Pt0.9Pd0.1)3P

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8.1Pressure unresolvedonset
SrPt3P

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8.4Pressure not reportedunknown
CaPt3P

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6.6Pressure not reportedunknown
LaPt3P

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

1.5Pressure not reportedunknown
MgCNi3

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

8Pressure not reportedunknown
CuNNi3

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

3.2Pressure not reportedunknown
SnSr3O

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

5Pressure not reportedunknown

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