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Effect of hydrostatic pressure on the unconventional charge density wave and superconducting properties in two distinct phases of doped kagome superconductors CsV3−xTixSb5

J. Hou, K. Y. Chen, J. P. Sun, Z. Zhao, Y. H. Zhang, P. F. Shan, N. N. Wang, H. Zhang, K. Zhu, Y. Uwatoko, H. Chen, H. T. Yang, X. L. Dong, H.-J. Gao, J.-G. Cheng

DOI 10.1103/PhysRevB.107.144502 · Physical Review B

T1

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Abstract

Recent studies on the kagome metal CsV3Sb5 have revealed an intricate interplay between unconventional charge density waves (CDWs) and superconductivity (SC). Substitutions of Ti for V can perturb the CDW and produce two distinct SC phases with different pairing symmetries in the series of CsV3−xTixSb5. Here, we performed a comprehensive high-pressure study on Ti-doped CsV3−xTixSb5 (x=0.04,0.15) samples to elucidate the combined effects of physical pressure and chemical doping on the coexistence of CDWs and SC. Under high pressures, the M-shaped double superconducting dome observed in the parent CsV3Sb5 is retained but very weakened for x=0.04, and it is replaced by a single broad superconducting dome for x=0.15. Accordingly, the optimal superconducting Tc under high pressures decreases gradually with increasing Ti-doping level. On the other hand, the upper critical field first exhibits an obvious rise with enhanced flux pinning effects by disorders for x=0.04 and then is suppressed upon further increasing Ti doping. The constructed T−P phase diagrams of CsV3−xTixSb5 reveal the competition and coexistence of CDWs and SC. Our results provide more insight into the intertwined competing electronic orders in the Ti-doped kagome superconductors CsV3−xTixSb5.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
CsV3Sb5

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2.5Pressure unresolvedunknown
CsV3Sb5

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3.8Pressure unresolvedonset
CsV3Sb5

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2.8Pressure unresolvedzero_resistance
CsV2.96Ti0.04Sb5

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2.9Pressure unresolvedonset
CsV2.96Ti0.04Sb5

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1.65Pressure unresolvedzero_resistance
CsV2.96Ti0.04Sb5

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7.91.66 GPaonset
CsV2.96Ti0.04Sb5

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7.651.66 GPazero_resistance
CsV2.85Ti0.15Sb5

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3.8Pressure unresolvedonset
CsV2.85Ti0.15Sb5

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2.4Pressure unresolvedzero_resistance
CsV2.85Ti0.15Sb5

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6.31.5 GPaonset
CsV2.85Ti0.15Sb5

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6.11.5 GPazero_resistance
CsV2.85Ti0.15Sb5

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6.31.5 GPaunknown

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