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Large upper critical fields and dimensionality crossover of superconductivity in the infinite-layer nickelate La0.8Sr0.2NiO2

Wei Wei, Wenjie Sun, Yue Sun, Yongqiang Pan, Gangjian Jin, Feng Yang, Yueying Li, Zengwei Zhu, Yuefeng Nie, Zhixiang Shi

DOI 10.1103/PhysRevB.107.L220503 · Physical Review B

T1

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Abstract

The recently emerging superconductivity in infinite-layer nickelates with the isostructural and isoelectronic characteristics of cuprates provides a new platform to explore the pairing mechanism of high-temperature superconductors. In this work, we studied the upper critical field (Hc2) of a high-quality La0.8Sr0.2NiO2 thin film with superconducting transition temperature, Tconset=18.8 K, using high magnetic field up to 56 T. A very large Hc2, ∼40 T for H∥c and ∼52 T for H⊥c, was confirmed, which suggests that infinite-layer nickelates also have great application potential. The anisotropy of Hc2 monotonically decreases from ∼10(γ=Hc2ab/Hc2c) near Tc to ∼1.5 at 2 K. Angle dependence of Hc2 confirms the crossover of superconductivity from two-dimensional to three-dimensional as the temperature decreases. We discussed that the interstitial orbital effect causes the weakening of anisotropy. The observed abnormal upturning of Hc2 at low temperatures is found to be a universal behavior independent of film quality and rare-earth elements. Therefore, it should not be the Fulde-Ferrell-Larkin-Ovchinnikov state due to the fact that it is in the dirty limit and insensitive to disorder.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
La0.8Sr0.2NiO2

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18.8Pressure not reportedonset
La0.8Sr0.2NiO2

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17.7Pressure not reportedmidpoint
Nd0.775Sr0.225NiO2

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8.5Pressure not reportedunknown
La0.8Sr0.2NiO2

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6.15Pressure not reportedunknown

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