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Evidence of unconventional vortex states in the Chevrel phase superconductor PbMo6Se8

Souvik Banerjee, Sudip Ghosh, Anshu Kataria, A. Sundaresan

DOI 10.1103/PhysRevB.110.014512 · Physical Review B

T1

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Abstract

We present a comprehensive investigation of superconducting properties in the Chevrel phase compound PbMo6Se8 by x-ray diffraction, dc magnetization, resistivity, heat capacity, and magnetic relaxation experiments. We determine a bulk superconducting transition temperature Tc of 3.8 K. Key superconducting parameters such as lower [μ0Hc1(0)] and upper [μ0Hc2(0)] critical fields, coherence length [ξGL(0)], penetration depth [λGL(0)], Ginzburg-Landau parameter (κ), Pauli paramagnetic field (μ0HPstr), and Maki parameter (αM) are obtained. The BCS model provides a reasonable description of the heat-capacity data. An unconventional vortex state is evident from the investigation of the unusual fishtail effect and nonmonotonous magnetic field dependency of the vortex pinning energy obtained from the magnetic relaxation experiments, indicating a deviation from the ideal type II superconducting vortex, in PbMo6Se8. A detailed μ0H-T phase diagram has been drawn illustrating a multiphase vortex crossover.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
PbMo6Se8

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3.8Pressure not reportedunknown
PbMo6Se8

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

4.2Pressure not reportedonset
PbMo6Se8

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4.11Pressure not reportedmidpoint
PbMo6S8

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—Pressure not reportedunknown
SnMo6S8

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

—Pressure not reportedunknown

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