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Continuously evolving antiferromagnetic order within the superconducting phase in Zn-doped CeCoIn5

Kaede Inoh, Ryosuke Koizumi, Teppei Takahashi, Hayao Fujimoto, Hideaki Ebisawa, Azumi Yashiro, Mika Kohinata, Asuka Hosogai, Akira Matsuo, Koichi Kindo, Ikuto Kawasaki, Daisuke Okuyama, Hung-Cheng Wu, Taku J. Sato, Kenichi Tenya, Kenji Ohoyama, Kazuaki Iwasa, Makoto Yokoyama

DOI 10.1103/PhysRevB.111.104510 · Physical Review B

T1

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Abstract

The antiferromagnetic (AFM) order inside the superconducting (SC) phase of CeCo(In1−xZnx)5 (x≤0.06) is investigated by neutron scattering, specific heat, and ac magnetic susceptibility measurements. It is confirmed that the AFM order with a modulation vector of q0=(1/2,1/2,1/2) develops for x>0.03, accompanied by the reduction of the SC transition temperature Tc from 2.3 K (x=0) to 1.6 K (x=0.06). The AFM transition temperature TN and the staggered moment μ continuously increase from zero within the SC phase as x increases beyond 0.03. For the small x range satisfying the TN<Tc condition, the AFM Bragg peak intensity shows an unusually gradual development with a (TN−T)2 function below TN and the specific heat shows no anomaly at TN. In contrast, when TN is larger than Tc at x=0.06, the AFM Bragg peak evolves with the conventional (TN−T) dependence and a clear jump in the specific heat occurs at TN. A coupling between the SC and AFM orders at the microscopic level is suggested to yield these unusual features observed in the small x range.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
CeCoIn5

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2.3Pressure not reportedonset
CeCo(In1-xZnx)5

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

1.6Pressure not reportedonset
CeCo(In1-xZnx)5

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

1.6Pressure not reportedonset

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