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Effect of magnetic impurities on high-temperature superconductivity in La1.85Sr0.15CuO4

G. W. Crabtree, W. K. Kwok, A. Umezawa, L. Soderholm, L. Morss, E. E. Alp

DOI 10.1103/PhysRevB.36.5258 · Physical Review B

T1

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Abstract

We have investigated the effect of magnetic impurities on the two-dimensional high-Tc superconductor La1.85Sr0.15CuO4 by replacing La with Nd. We find a decrease in Tc and dHc2dT|Tc and an increase in the normal-state resistivity with increasing Nd content. We use the Werthamer, Helfand, and Hohenberg equations to derive the effect of an exchange field, magnetic polarization, nonmagnetic impurity scattering, and changes in the density of states on Tc and dHc2dT|Tc. We find no evidence of an exchange interaction between the magnetic moments and the conduction electrons. We explain the changes in the superconducting properties in terms of the van Hove singularity in the density of states near the Fermi level.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
La1.85Sr0.15CuO4

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37Pressure not reportedonset
La1.85Sr0.15CuO4

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34.4Pressure not reportedmidpoint
La1.85Sr0.15CuO4

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24Pressure not reportedzero_resistance
La1.82Nd0.03Sr0.15CuO4

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

38Pressure not reportedonset
La1.82Nd0.03Sr0.15CuO4

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

34.2Pressure not reportedmidpoint
La1.82Nd0.03Sr0.15CuO4

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

28Pressure not reportedzero_resistance
La1.45Nd0.4Sr0.15CuO4

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

30Pressure not reportedonset
La1.45Nd0.4Sr0.15CuO4

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

22.5Pressure not reportedmidpoint
La1.45Nd0.4Sr0.15CuO4

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

9Pressure not reportedzero_resistance

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