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Suppression of superconductivity by antiferromagnetism in Tm2Fe3Si5

J. A. Gotaas, J. W. Lynn, R. N. Shelton, P. Klavins, H. F. Braun

DOI 10.1103/PhysRevB.36.7277 · Physical Review B

T1

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Abstract

Powder neutron-diffraction experiments at pressures up to 8.2 kbar and temperatures down to 0.3 K have been performed on the antiferromagnetic ternary compound Tm2Fe3Si5. For pressures between 2 and 21 kbar, this system becomes superconducting at Tc1>TN, with a subsequent reentrance to the normal conducting state at Tc2≈TN. Our measurements demonstrate that the antiferromagnetic structure is unchanged under pressure, with no evidence for a ferromagnetic component at any pressure that would compete with the superconducting phase. This is the first experimental observation of the quenching of superconductivity by a purely antiferromagnetic state.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
Tm2Fe3Si5

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3.50.82 GPaonset
Tm2Fe3Si5

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

3.50.82 GPaonset

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