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Use of Kramers-Kronig relations to extract the conductivity of high-Tc superconductors from optical data

D. Miller, P. L. Richards

DOI 10.1103/PhysRevB.47.12308 · Physical Review B

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Abstract

In principle the conductivity of the cuprate superconductors can be obtained from reflectivity measurements using the Kramers-Kronig-transform technique. However, at low temperatures and for frequencies below ∼300 cm−1 the reflectivities of materials such as YBa2Cu3O7 are close to unity. Uncertainty in the precise signal level corresponding to unity reflectivity and a lack of knowledge of the reflectivity below the lowest measured frequency cause this method to become unreliable. To address this problem we have used a bolometric technique and a resonant technique to obtain accurate submillimeter and microwave data for the residual losses in epitaxial thin films of YBa2Cu3O7 at low temperatures. The Kramers-Kronig analysis of our data is in good agreement with results from fitting our data to simple weakly coupled grain and two-fluid models for the a-b plane conductivity. However, below 450 cm−1 it is in disagreement with some published results of other workers obtained from Kramers-Kronig analysis of reflectivity data. To understand this discrepancy we analyze how the conductivity determined by the Kramers-Kronig-transform technique depends on some commonly used low-frequency extrapolations of reflectivity data.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
YBa2Cu3O7

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—Pressure not reportedunknown

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