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Two-magnon Raman scattering in cuprate superconductors: Evolution of magnetic fluctuations with doping

G. Blumberg, R. Liu, M. V. Klein, W. C. Lee, D. M. Ginsberg, C. Gu, B. W. Veal, B. Dabrowski

DOI 10.1103/PhysRevB.49.13295 · Physical Review B

T1

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Abstract

We report observation and resonance Raman studies of spin-pair excitations in YBa2Cu3O6+x (0.37<x<0.7) and YBa2Cu4O8 superconductors. These excitations at energy ∼3J (2700±150 cm−1), similar to two-magnon excitations in insulators, are evidence that antiferromagnetic fluctuations with spatial extent of at least three lattice constants are not overdamped in the underdoped superconductors. With optimal hole dopings, where Tc>80 K, the two-magnon peak can no longer be seen above the flat Raman continuum. Photoluminescence and the origin of the broad-spectrum Raman continuum are also discussed.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
YBa2Cu3O6+x

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13Pressure not reportedunknown
YBa2Cu3O6+x

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

70Pressure not reportedunknown
YBa2Cu3O6+x

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

92Pressure not reportedunknown
YBa2Cu3O6+x

Archive — visibility unverified

Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

60Pressure not reportedunknown
YBa2Cu3O6+x

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

90Pressure not reportedunknown
YBa2Cu4O8

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

80Pressure not reportedunknown