Two types of magnetism in the magnetic superconductor TmNi2B2C related to the degree of carbon-site occupancy
A. M. Mulders, P. C. M. Gubbens, U. Gasser, C. Baines, K. H. J. Buschow
DOI 10.1103/PhysRevB.57.10320 · Physical Review B
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Abstract
A combined 169Tm Mössbauer spectroscopy and μ+SR (muon spin rotation) study is presented on a polycrystalline sample of TmNi2B2C. The first experimental technique shows the coexistence of two types of Tm 4f magnetism at 0.3 K, one related to a magnetic Tm moment of 4.3(1)μB and the other to a small Tm moment of ∼0.1μB. This second type of magnetism is suggested to be caused by carbon vacancies present in TmNi2B2C. These C vacancies locally modify the crystalline electric field and therefore the Tm 4f magnetism. Since these vacancies are ideal cavities in which muons can reside, it is suggested that μ+SR only probes this ∼0.1μB magnetism.
Source-reported materials — not catalogue approval
| Formula | Reported Tc (K) | Pressure (GPa) | Type |
|---|---|---|---|
| TmNi2B2C Archive — visibility unverified Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula. | 10.3 | Pressure not reported | unknown |
| TmNi2B2C Archive — visibility unverified Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula. | 10.8 | Pressure not reported | unknown |
| DyNi2B2C Archive — visibility unverified Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula. | 6 | Pressure not reported | unknown |
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