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Superconducting fluctuations and anomalous diamagnetism in underdoped YBa2Cu3O6+x from magnetization and 63Cu NMR-NQR relaxation measurements

P. Carretta, A. Lascialfari, A. Rigamonti, A. Rosso, A. Varlamov

DOI 10.1103/PhysRevB.61.12420 · Physical Review B

T1

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Abstract

Magnetization and 63Cu nuclear magnetic resonance-nuclear quadrupole resonance relaxation measurements are used to study the superconducting fluctuations in YBa2Cu3O6+x (YBCO) oriented powders. In optimally doped YBCO the fluctuating negative magnetization Mfl(H,T) is rather well described by an anisotropic Ginzburg-Landau (GL) functional and the curves Mfl/H cross at Tc. In underdoped YBCO, instead, over a wide temperature range an anomalous diamagnetism is observed, stronger than in the optimally doped compound by about an order of magnitude. The field and temperature dependence of Mfl cannot be described either by an anisotropic GL functional or on the basis of scaling arguments. The anomalous diamagnetism is more pronounced in samples with a defined order in the Cu(1)O chains. The 63Cu(2) relaxation rate shows little, if any, field dependence in the vicinity of the transition temperature Tc(H=0). It is argued how the results in the underdoped compounds can be accounted for by the presence of charge inhomogeneities, favored by chains ordering.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
YBa2Cu3O6+x

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91.1Pressure unresolvedzero_resistance
YBa2Cu3O6+x

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

64.5Pressure unresolvedzero_resistance
YBa2Cu3O6+x

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64.2Pressure unresolvedzero_resistance
YBa2Cu4O8

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—Pressure not reportedunknown

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