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Effect of pressure on the superconducting and spin-density-wave states of SmFeAsO1−xFx

B. Lorenz, K. Sasmal, R. P. Chaudhury, X. H. Chen, R. H. Liu, T. Wu, C. W. Chu

DOI 10.1103/PhysRevB.78.012505 · Physical Review B

T1

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Abstract

High-temperature superconductors with a Tc above 40 K have been found to be strongly correlated electron systems and to have a layered structure. Guided by these rules, Kamihara et al. [J. Am. Chem. Soc. 130, 3296 (2008)] discovered a Tc up to 26 K in the layered La(O1−xFx)FeAs. By replacing La with trivalence rare-earth (RE) elements of smaller ionic radii, Tc has subsequently been raised to 41–52 K. Many theoretical models have been proposed that emphasize the important magnetic origin of superconductivity in this compound system and a possible further Tc enhancement in RE(O1−xFx)FeAs by compression. This later prediction appears to be supported by the pressure-induced Tc increase in La(O0.89F0.11)FeAs observed. Here we show that, in contrast to previous expectations, pressure can either suppress or enhance Tc, depending on the doping level, suggesting that a Tc exceeding 50 K may be found only in the yet-to-be discovered compound systems related to but different from RE(O1−xFx)FeAs and that the Tc of La(O1−xFx)FeAs and Sm(O1−xFx)FeAs may be further raised to about 50 K.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
La(O1-xFx)FeAs

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26Pressure not reportedunknown
LaOFeP

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4Pressure not reportedunknown
LaONiP

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3Pressure not reportedunknown
Sm(O1-xFx)FeAs

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43Pressure not reportedunknown
Ce(O1-xFx)FeAs

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41Pressure not reportedunknown
Pr(O1-xFx)FeAs

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52Pressure not reportedunknown
Nd(O1-xFx)FeAs

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50Pressure not reportedunknown
YBa2Cu3O7

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93Pressure not reportedunknown
Sm(O0.7F0.3)FeAs

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48Pressure unresolvedonset
Sm(O0.87F0.13)FeAs

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30Pressure unresolvedonset
Sm(O0.87F0.13)FeAs

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24.7Pressure unresolvedmidpoint
Sm(O0.87F0.13)FeAs

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25.550.94 GPamidpoint

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