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Strong-coupling superconductivity in the nickel-based oxypnictide LaNiAsO1−xFx

Zheng Li, Gengfu Chen, Jing Dong, Gang Li, Wanzheng Hu, Dan Wu, Shaokui Su, Ping Zheng, Tao Xiang, Nanlin Wang, Jianlin Luo

DOI 10.1103/PhysRevB.78.060504 · Physical Review B

T1

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Abstract

A series of layered nickel-based LaNiAsO1−xFx compounds with x=0–0.15 are synthesized by solid-state reactions. The pure LaNiAsO exhibits bulk superconductivity with Tc∼2.75 K. Partial substitution of oxygen with fluorine increases the transition temperature to ∼3.8 K. The LaNiAsO0.9F0.1 sample shows a sharp superconducting transition and a sharp specific-heat jump at the critical temperature. The magnitude of the specific-heat jump is much larger than that expected from the weak-coupling BCS theory, indicating that this superconductor is in the strong-coupling regime. Furthermore, the temperature dependence of the specific heat deviates strongly from the theoretical result for the single-band s- or d-wave superconductor but shows a characteristic feature of multigap.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
LaNiAsO

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2.75Pressure not reportedonset
LaNiAsO

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1.8Pressure not reportedonset
LaNiAsO0.9F0.1

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3.8Pressure not reportedonset
LaNiAsO0.9F0.1

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3.8Pressure not reportedonset
LaNiAsO0.94F0.06

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3.78Pressure not reportedunknown
LaFePO

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4Pressure not reportedunknown
LaNiPO

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3Pressure not reportedunknown
LaFeAsO1-xFx

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26Pressure not reportedunknown

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