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Coexistence of superconductivity and antiferromagnetic ordering in the layered superconductor SmFePO

Yoichi Kamihara, Hidenori Hiramatsu, Masahiro Hirano, Yasuhiro Kobayashi, Shinji Kitao, Satoshi Higashitaniguchi, Yoshitaka Yoda, Makoto Seto, Hideo Hosono

DOI 10.1103/PhysRevB.78.184512 · Physical Review B

T1

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Abstract

Superconductivity and magnetic transition in SmFePO were examined by electric, magnetic, F57e Mössbauer, and S149m nuclear resonant forward-scattering (NRFS) measurements. Zero resistivity and negative magnetic susceptibility were observed in an undoped SmFePO, indicating superconducting transition temperature (Tc) of ∼3 K. Tc in undoped SmFePO appears in a narrow region of lattice constants with an optimum conductivity. Furthermore, in relation to magnetic susceptibility, NRFS spectra verify that magnetic moments of Sm3+ ions order antiferromagnetically below magnetic transition ∼5 K, accompanying a discontinuous drop in electrical resistivity, whereas F57e Mössbauer spectra show that magnetic moments of Fe are quenched. These results indicate the coexistence of superconductivity and magnetic ordering in a crystallographic unit cell of SmFePO.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
SmFePO

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3Pressure not reportedmidpoint
SmFePO

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3Pressure not reportedonset
LaFePO

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2.4Pressure not reportedunknown

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