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Annealing effect on the electron-doped superconductor Pr0.88LaCe0.12CuO4±δ

Yong-Lei Wang, Yan Huang, Lei Shan, S. L. Li, Pengcheng Dai, Cong Ren, Hai-Hu Wen

DOI 10.1103/PhysRevB.80.094513 · Physical Review B

T1

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Abstract

Using high-vacuum annealing treatment, the superconducting transition temperature Tc of the electron-doped Pr0.88LaCe0.12CuO4±δ single crystals was successfully driven to a regime in which the Tc value continuously decreases with oxygen removal. This regime of oxygen-reduction process is hard to be understood according to the previous knowledge of this material. In addition, a remarkable relaxation of Tc over time was observed at room temperature, indicating that the variation in Tc is closely related to the rearrangement of oxygen in the sample. In combination with previous studies, it can be concluded that, in the whole process of oxygen reduction applied on Pr0.88LaCe0.12CuO4±δ, although the strength of antiferromagnetic (fluctuation) correlations does play a role, Tc is dominated by the disorder effect of CuO2 plane either on copper sites or oxygen sites, which leads to a strong depairing effect.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
Pr0.88LaCe0.12CuO4±δ

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25.9Pressure not reportedonset
Pr0.88LaCe0.12CuO4±δ

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23Pressure not reportedonset
Pr0.88LaCe0.12CuO4±δ

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23.2Pressure not reportedonset
Nd2-xCexCuO4±δ

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—Pressure not reportedunknown
Pr2-xCexCuO4±δ

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—Pressure not reportedunknown
YBa2Cu3O7-δ

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—Pressure not reportedunknown

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