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Electron-phonon coupling and the charge gap of spin-density wave iron-pnictide materials from quasiparticle relaxation dynamics

L. Stojchevska, P. Kusar, T. Mertelj, V. V. Kabanov, X. Lin, G. H. Cao, Z. A. Xu, D. Mihailovic

DOI 10.1103/PhysRevB.82.012505 · Physical Review B

T1

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Abstract

We investigate the quasiparticle relaxation and low-energy electronic structure in undoped SrFe2As2 exhibiting spin-density wave (SDW) ordering using optical pump-probe femtosecond spectroscopy. A remarkable critical slowing down of the quasiparticle relaxation dynamics at the SDW transition temperature TSDW=200 K is observed. From temperature dependence of the transient reflectivity amplitude we determine the SDW-state charge gap magnitude, 2ΔSDW/kBTSDW=7.2±1. The second moment of the Eliashberg function, λ⟨(ℏω)2⟩=110±10 meV2, determined from the relaxation time above TSDW, is similar to SmFeAsO and BaFe2As2 indicating a moderate electron phonon coupling.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
SrFe2As2

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

—Pressure not reportedunknown
SmFeAsO

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

—Pressure not reportedunknown
BaFe2As2

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

—Pressure not reportedunknown

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