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Superconductivity and magnetic properties of single crystals of K0.75Fe1.66Se2 and Cs0.81Fe1.61Se2

J. J. Ying, X. F. Wang, X. G. Luo, A. F. Wang, M. Zhang, Y. J. Yan, Z. J. Xiang, R. H. Liu, P. Cheng, G. J. Ye, X. H. Chen

DOI 10.1103/PhysRevB.83.212502 · Physical Review B

T1

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Abstract

We successfully grew the high-quality single crystals of AxFe2Se2 (A = K and Cs) by self-flux method. Sharp superconducting transition was observed for both types of crystals. The crystals show the onset superconducting transition temperatures (Tc) of 31 and 30 K for K and Cs compounds, respectively, with nearly 100% superconductive shielding fraction. The crystals show quite high resistivity in the normal state of more than 160 and 1300 mΩ cm maximum resistivity for KxFe2Se2 and CsxFe2Se2 single crystals, respectively. Much larger upper critical field Hc2 is inferred from low-temperature isomagnetic-field magnetoresistance in these crystals than in FeSe. The anisotropy Hc2ab(0)/Hc2c(0) is estimated to be around 3 for both of the two materials. Anisotropic peculiar magnetic behavior in normal state has been found for CsxFe2Se2

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
K0.75Fe1.66Se2

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31Pressure unresolvedonset
K0.75Fe1.66Se2

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28.7Pressure unresolvedzero_resistance
K0.75Fe1.66Se2

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29Pressure unresolvedonset
Cs0.81Fe1.61Se2

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30Pressure unresolvedonset
Cs0.81Fe1.61Se2

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26.5Pressure unresolvedzero_resistance
Cs0.81Fe1.61Se2

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25.5Pressure unresolvedonset
LaFeAs(O,F)

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26Pressure not reportedunknown
FeSe

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8Pressure unresolvedunknown
FeSe

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374.5 GPaonset

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