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Two-magnon Raman scattering in A0.8Fe1.6Se2 systems (A=K, Rb, Cs, and Tl): Competition between superconductivity and antiferromagnetic order

A. M. Zhang, J. H. Xiao, Y. S. Li, J. B. He, D. M. Wang, G. F. Chen, B. Normand, Q. M. Zhang, T. Xiang

DOI 10.1103/PhysRevB.85.214508 · Physical Review B

T1

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Abstract

We performed Raman-scattering measurements on high-quality single crystals of A0.8Fe1.6Se2 superconductors of several compositions. We found a broad, asymmetric peak around 1600 cm−1 (200 meV), which we identify as a two-magnon process involving optical magnons. The intensity of the two-magnon peak falls sharply on entering the superconducting phase. This effect, which is entirely absent in the non-superconducting system KFe1.5Se2, requires a strong mutual exclusion between antiferromagnetism and superconductivity arising from proximity effects within regions of microscale phase separation.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
K0.8Fe1.6Se2

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32Pressure not reportedunknown
K0.8Fe1.6Se2

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32Pressure not reportedunknown
Tl0.5K0.3Fe1.6Se2

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29Pressure not reportedunknown
Tl0.5K0.3Fe1.6Se2

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29Pressure not reportedunknown
Tl0.5Rb0.3Fe1.6Se2

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31Pressure not reportedunknown
Tl0.5Rb0.3Fe1.6Se2

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31Pressure not reportedunknown

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