Fractional power-law behavior and its origin in iron-chalcogenide and ruthenate superconductors: Insights from first-principles calculations

Z. P. Yin; K. Haule; G. Kotliar

doi:10.1103/PhysRevB.86.195141

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Fractional power-law behavior and its origin in iron-chalcogenide and ruthenate superconductors: Insights from first-principles calculations

Z. P. Yin, K. Haule, G. Kotliar

DOI 10.1103/PhysRevB.86.195141 · Physical Review B

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Abstract

We perform realistic first-principles calculations of iron chalcogenides and ruthenate-based materials to identify experimental signatures of Hund's-coupling-induced correlations in these systems. We find that FeTe and KxFe2−ySe2 display unusual orbital-dependent fractional power-law behavior in their quasiparticle self-energy and optical conductivity, a phenomenon first identified in SrRuO3. Strong incoherence in the paramagnetic state of these materials results in electronic states hidden to angle-resolved photoemission spectroscopy which reemerge at low temperatures. We identify the effective low-energy Hamiltonian describing these systems and show that these anomalies are not controlled by the proximity to a quantum critical point but result from coexistence of fast quantum mechanical orbital fluctuations and slow spin fluctuations.