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Photoemission and muon spin relaxation spectroscopy of the iron-based Rb0.77Fe1.61Se2 superconductor: Crucial role of the cigar-shaped Fermi surface

J. Maletz, V. B. Zabolotnyy, D. V. Evtushinsky, A. N. Yaresko, A. A. Kordyuk, Z. Shermadini, H. Luetkens, K. Sedlak, R. Khasanov, A. Amato, A. Krzton-Maziopa, K. Conder, E. Pomjakushina, H.-H. Klauss, E. D. L. Rienks, B. Büchner, S. V. Borisenko

DOI 10.1103/PhysRevB.88.134501 · Physical Review B

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Abstract

In this study, we investigate the electronic and magnetic properties of Rb0.77Fe1.61Se2 (Tc = 32.6 K) in normal and superconducting states by means of photoemission and μSR spectroscopies as well as band-structure calculations. We demonstrate that the unusual behavior of these materials is the result of separation into metallic (∼12%) and insulating (∼88%) phases. Only the former becomes superconducting and has a usual electronic structure of electron-doped FeSe slabs. Our results thus imply that the antiferromagnetic insulating phase is just a by-product of Rb intercalation and its magnetic properties have no direct relation to the superconductivity. Instead, we find that also in this class of iron-based compounds, the key ingredient for superconductivity is a certain proximity of a Van Hove singularity to the Fermi level.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
Rb0.77Fe1.61Se2

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32.6Pressure not reportedunknown
Rb0.77Fe1.61Se2

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32.6Pressure not reportedunknown
FeSe

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—1.9 GPaunknown

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