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Weak phonon-mediated pairing in BiS2 superconductor from first principles

Corentin Morice, Ryosuke Akashi, Takashi Koretsune, Siddharth S. Saxena, Ryotaro Arita

DOI 10.1103/PhysRevB.95.180505 · Physical Review B

T1

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Abstract

Superconductivity in novel bismuth-sulfur superconductors has attracted large research efforts, both experimental and theoretical, but a consensus on the nature of superconductivity in these materials has yet to be reached. Using density functional theory for superconductors, we study the electron-phonon pairing mechanism in LaO0.5F0.5BiS2. We first confirm the presence of a commensurate charge density wave instability, in accordance with previous studies. Using a recently developed integration scheme for the electron-phonon coupling, we found that its strength is much lower than previously calculated, due to improved density of states calculations. We finally conclude that conventional phonon-mediated pairing cannot explain the high superconducting transition temperatures observed in this material.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
LaO0.5F0.5BiS2

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—Pressure not reportedunknown
La(O,F)BiS2

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

10.6Pressure not reportedunknown

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