Observation of a crossover from nodal to gapped superconductivity in LuxZr1−xB12
Franziska K. K. Kirschner, Nikolay E. Sluchanko, Vladimir B. Filipov, Francis L. Pratt, Chris Baines, Natalya Yu. Shitsevalova, Stephen J. Blundell
DOI 10.1103/PhysRevB.98.094505 · Physical Review B
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Abstract
We have determined the superconducting and magnetic properties of four samples of LuxZr1−xB12 (x=0.04, 0.07, 0.17, and 0.8) using muon spin rotation (μSR) and magnetometry measurements. We observed a strong magnetic signal in both the μSR and magnetometry data in one sample (x=0.07), likely caused by the formation of static moments of size ≈1μB due to a clustering effect of the Lu3+ ions. In all other samples, we find only a small magnetic signal in the μSR data thought to originate from boron nuclei in the B12 cages. The superconductivity is found to evolve with x, with a decrease in x resulting in an increase in critical temperature and a decrease of the penetration depth. Most remarkably, we find evidence for the formation of nodes in the superconducting gap for x≤0.17, providing a potential new example of an s-to-s+d-wave crossover in a superconductor.
Source-reported materials — not catalogue approval
| Formula | Reported Tc (K) | Pressure (GPa) | Type |
|---|---|---|---|
| LuxZr1-xB12 Archive — visibility unverified Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula. | — | Pressure not reported | unknown |
| ZrB12 Archive — visibility unverified Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula. | 6 | Pressure not reported | unknown |
| LuB12 Archive — visibility unverified Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula. | 0.48 | Pressure not reported | unknown |
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