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Anisotropic superconductivity and magnetism in single-crystal RbEuFe4As4

M. P. Smylie, K. Willa, J.-K. Bao, K. Ryan, Z. Islam, H. Claus, Y. Simsek, Z. Diao, A. Rydh, A. E. Koshelev, W.-K. Kwok, D. Y. Chung, M. G. Kanatzidis, U. Welp

DOI 10.1103/PhysRevB.98.104503 · Physical Review B

T1

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Abstract

We investigate the anisotropic superconducting and magnetic properties of single-crystal RbEuFe4As4 using magnetotransport and magnetization measurements. We determine a magnetic ordering temperature of the Eu moments of Tm=15K and a superconducting transition temperature of Tc=36.8K. The superconducting phase diagram is characterized by high upper critical field slopes of −70 and −42 kG/K for in-plane and out-of-plane fields, respectively, and a surprisingly low superconducting anisotropy of Γ=1.7. Ginzburg-Landau parameters of κc∼67 and κab∼108 indicate extreme type-II behavior. These superconducting properties are in line with those commonly seen in optimally doped Fe-based superconductors. In contrast, Eu magnetism is quasi-two dimensional (2D), as evidenced by highly anisotropic in-plane and out-of-plane exchange constants of 0.6 K and <0.04 K. A consequence of the quasi-2D nature of the Eu magnetism are strong magnetic fluctuation effects, a large suppression of the magnetic ordering temperature as compared to the Curie-Weiss temperature, and a kinklike anomaly in the specific heat devoid of any singularity. Magnetization curves reveal a clear magnetic easy-plane anisotropy with in-plane and out-of-plane saturation fields of 2 and 4 kG.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
RbEuFe4As4

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36.8Pressure not reportedunknown
RbEuFe4As4

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36.8Pressure not reportedonset
CsEuFe4As4

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37Pressure not reportedunknown
CaKFe4As4

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35Pressure not reportedunknown
(La,Na)(Cs,Rb)Fe4As4

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25Pressure not reportedunknown

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