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Spin Dynamics in Iron-Based Layered Superconductor (La0.87Ca0.13)FePO Revealed by P31 and La139 NMR Studies

Yusuke Nakai, Kenji Ishida, Yoichi Kamihara, Masahiro Hirano, Hideo Hosono

DOI 10.1103/PhysRevLett.101.077006 · Physical Review Letters

T1

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Abstract

We report P31 and La139 NMR studies of (La0.87Ca0.13)FePO, which is a family member of the recently discovered superconductor LaFeAs(O1−xFx). In the normal state, Knight shift and nuclear spin-lattice relaxation rate divided by T (1/T1T) show that a Fermi-liquid state with moderate ferromagnetic fluctuations emerges below 30 K. From 1/T1T of P31 and La139, a quasi-two- dimensional electronic structure is suggested, in which the FeP layer is more conductive than the LaO layer. In the superconducting (SC) state, although a clear Meissner signal was observed, 1/T1T increases below Tc, in contrast to a decrease of 1/T1T due to the opening of a SC gap, suggesting that novel low-energy spin dynamics develop in the SC state.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
(La0.87Ca0.13)FePO

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8Pressure not reportedonset
(La0.87Ca0.13)FePO

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8Pressure not reportedonset
(La0.87Ca0.13)FePO

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5.9Pressure not reportedmidpoint
LaFeAs(O1-xFx)

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26Pressure not reportedunknown
SmFeAs(O1-xFx)

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55Pressure not reportedunknown
LaFePO

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4Pressure not reportedunknown

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