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Unusual Layer-Dependent Charge Distribution, Collective Mode Coupling, and Superconductivity in Multilayer Cuprate Ba2Ca3Cu4O8F2

Yulin Chen, Akira Iyo, Wanli Yang, Akihiro Ino, M. Arita, Steve Johnston, Hiroshi Eisaki, H. Namatame, M. Taniguchi, Thomas P. Devereaux, Zahid Hussain, Z.-X. Shen

DOI 10.1103/PhysRevLett.103.036403 · Physical Review Letters

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Abstract

Low energy ultrahigh momentum resolution angle resolved photoemission spectroscopy study on four-layer self-doped high Tc superconductor Ba2Ca3Cu4O8F2 (F0234) revealed fine structure in the band dispersion, identifying the unconventional association of hole and electron doping with the inner and outer CuO2 layers, respectively. For the states originating from two inequivalent CuO2 layers, different energy scales are observed in dispersion kinks associated with the collective mode coupling, with the larger energy scale found in the electron (n-) doped state which also has stronger coupling strength. Given the earlier finding that the superconducting gap is substantially larger along the n-type Fermi surface, our observations connect the mode coupling energy and strength with magnitude of the pairing gap.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
Ba2Ca3Cu4O8F2

Archive — visibility unverified

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—Pressure not reportedunknown
Bi2Sr2CaCu2O8

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

70Pressure not reportedunknown

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