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Angle-Dependent Evolution of the Fulde-Ferrell-Larkin-Ovchinnikov State in an Organic Superconductor

R. Beyer, B. Bergk, S. Yasin, J. A. Schlueter, J. Wosnitza

DOI 10.1103/PhysRevLett.109.027003 · Physical Review Letters

T1

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Abstract

We report magnetic-field and angular-dependent high-resolution specific-heat measurements of the organic superconductor β′′−(BEDT−TTF)2SF5CH2CF2SO3. When the magnetic field is aligned precisely within the conducting BEDT-TTF layer, at low temperatures a clear upturn of the upper critical field beyond the Pauli limit of 9.73 T is observed, hinting at the emergence of a Fulde-Ferrell-Larkin-Ovchinnikov state. This upturn disappears when the field is oriented out of plane by more than ∼0.5 deg. For smaller out-of-plane angles, the specific-heat anomaly at Tc sharpens and a second peaky phase transition appears within the superconducting state.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
(BEDT-TTF)2SF5CH2CF2SO3

Archive — visibility unverified

Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

4.3Pressure not reportedonset
(BEDT-TTF)2Cu(NCS)2

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

—Pressure not reportedunknown

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