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Pressure- and Composition-Induced Structural Quantum Phase Transition in the Cubic Superconductor (Sr,Ca)3Ir4Sn13

Lina E. Klintberg, Swee K. Goh, Patricia L. Alireza, Paul J. Saines, David A. Tompsett, Peter W. Logg, Jinhu Yang, Bin Chen, Kazuyoshi Yoshimura, F. Malte Grosche

DOI 10.1103/PhysRevLett.109.237008 · Physical Review Letters

T1

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Abstract

We show that the quasi-skutterudite superconductor Sr3Ir4Sn13 undergoes a structural transition from a simple cubic parent structure, the I phase, to a superlattice variant, the I′ phase, which has a lattice parameter twice that of the high temperature phase. We argue that the superlattice distortion is associated with a charge density wave transition of the conduction electron system and demonstrate that the superlattice transition temperature T* can be suppressed to zero by combining chemical and physical pressure. This enables the first comprehensive investigation of a superlattice quantum phase transition and its interplay with superconductivity in a cubic charge density wave system.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
Sr3Ir4Sn13

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5Pressure unresolvedonset
Sr3Ir4Sn13

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5Pressure unresolvedonset
Ca3Ir4Sn13

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7Pressure unresolvedunknown
Ca3Ir4Sn13

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7Pressure unresolvedunknown
Ca3Ir4Sn13

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8.94 GPaunknown

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