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Resonant X-Ray Scattering Measurements of a Spatial Modulation of the Cu 3d and O 2p Energies in Stripe-Ordered Cuprate Superconductors

A. J. Achkar, F. He, R. Sutarto, J. Geck, H. Zhang, Y.-J. Kim, D. G. Hawthorn

DOI 10.1103/PhysRevLett.110.017001 · Physical Review Letters

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Abstract

A prevailing description of the stripe phase in underdoped cuprate superconductors is that the charge carriers (holes) phase segregate on a microscopic scale into hole-rich and hole-poor regions. We report resonant elastic x-ray scattering measurements of stripe-ordered La1.475Nd0.4Sr0.125CuO4 at the Cu L and O K absorption edges that identify an additional feature of stripe order. Analysis of the energy dependence of the scattering intensity reveals that the dominant signature of the stripe order is a spatial modulation in the energies of Cu 3d and O 2p states rather than the large modulation of the charge density (valence) envisioned in the common stripe paradigm. These energy shifts are interpreted as a spatial modulation of the electronic structure and may point to a valence-bond-solid interpretation of the stripe phase.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
La1.475Nd0.4Sr0.125CuO4

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—Pressure not reportedunknown
La2-xBaxCuO4

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—Pressure not reportedunknown
La2-x-yEuySrxCuO4

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

—Pressure not reportedunknown
YBa2Cu3O6+δ

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—Pressure not reportedunknown
La2-xSrxCuO4

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—Pressure not reportedunknown

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