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Melting of Charge Stripes in Vibrationally Driven La1.875Ba0.125CuO4: Assessing the Respective Roles of Electronic and Lattice Order in Frustrated Superconductors

M. Först, R. I. Tobey, H. Bromberger, S. B. Wilkins, V. Khanna, A. D. Caviglia, Y.-D. Chuang, W. S. Lee, W. F. Schlotter, J. J. Turner, M. P. Minitti, O. Krupin, Z. J. Xu, J. S. Wen, G. D. Gu, S. S. Dhesi, A. Cavalleri, J. P. Hill

DOI 10.1103/PhysRevLett.112.157002 · Physical Review Letters

T1

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Abstract

We report femtosecond resonant soft x-ray diffraction measurements of the dynamics of the charge order and of the crystal lattice in nonsuperconducting, stripe-ordered La1.875Ba0.125CuO4. Excitation of the in-plane Cu-O stretching phonon with a midinfrared pulse has been previously shown to induce a transient superconducting state in the closely related compound La1.675Eu0.2Sr0.125CuO4. In La1.875Ba0.125CuO4, we find that the charge stripe order melts promptly on a subpicosecond time scale. Surprisingly, the low temperature tetragonal (LTT) distortion is only weakly reduced, reacting on significantly longer time scales that do not correlate with light-induced superconductivity. This experiment suggests that charge modulations alone, and not the LTT distortion, prevent superconductivity in equilibrium.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
La1.875Ba0.125CuO4

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3Pressure not reportedonset
La1.675Eu0.2Sr0.125CuO4

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

25Pressure not reportedunknown

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