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Impact of Atomic-Scale Contact Geometry on Andreev Reflection

J. Brand, P. Ribeiro, N. Néel, S. Kirchner, J. Kröger

DOI 10.1103/PhysRevLett.118.107001 · Physical Review Letters

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Abstract

Charge transport has been examined in junctions comprising the normal-metal tip of a low-temperature scanning tunneling microscope, the surface of a conventional superconductor, and adsorbed C60 molecules. The Bardeen-Cooper-Schrieffer energy gap gradually evolves into a zero-bias peak with decreasing electrode separation. The peak is assigned to the spectroscopic signature of Andreev reflection. The conductance due to Andreev reflection is determined by the atomic termination of the tip apex and the molecular adsorption orientation. Transport calculations unveil the finite temperature and the strong molecule-electrode hybridization as the origin to the surprisingly good agreement between spectroscopic data and the Blonder-Tinkham-Klapwijk model that was conceived for macroscopic point contacts.

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FormulaReported Tc (K)Pressure (GPa)Type
Nb

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9.21Pressure not reportedunknown
Nb

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9.2Pressure not reportedunknown
V3Si

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Pb

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—Pressure not reportedunknown

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