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Local Orthorhombicity in the Magnetic C4 Phase of the Hole-Doped Iron-Arsenide Superconductor Sr1−xNaxFe2As2

Benjamin A. Frandsen, Keith M. Taddei, Ming Yi, Alex Frano, Zurab Guguchia, Rong Yu, Qimiao Si, Daniel E. Bugaris, Ryan Stadel, Raymond Osborn, Stephan Rosenkranz, Omar Chmaissem, Robert J. Birgeneau

DOI 10.1103/PhysRevLett.119.187001 · Physical Review Letters

T1

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Abstract

We report on temperature-dependent pair distribution function measurements of Sr1−xNaxFe2As2, an iron-based superconductor system that contains a magnetic phase with reentrant tetragonal symmetry, known as the magnetic C4 phase. Quantitative refinements indicate that the instantaneous local structure in the C4 phase comprises fluctuating orthorhombic regions with a length scale of ∼2 nm, despite the tetragonal symmetry of the average static structure. Additionally, local orthorhombic fluctuations exist on a similar length scale at temperatures well into the paramagnetic tetragonal phase. These results highlight the exceptionally large nematic susceptibility of iron-based superconductors and have significant implications for the magnetic C4 phase and the neighboring C2 and superconducting phases.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
Sr1-xNaxFe2As2

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10Pressure not reportedunknown

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