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Fermiology and Superconductivity of Topological Surface States in PdTe2

O. J. Clark, M. J. Neat, K. Okawa, L. Bawden, I. Marković, F. Mazzola, J. Feng, V. Sunko, J. M. Riley, W. Meevasana, J. Fujii, I. Vobornik, T. K. Kim, M. Hoesch, T. Sasagawa, P. Wahl, M. S. Bahramy, P. D. C. King

DOI 10.1103/PhysRevLett.120.156401 · Physical Review Letters

T1

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Abstract

We study the low-energy surface electronic structure of the transition-metal dichalcogenide superconductor PdTe2 by spin- and angle-resolved photoemission, scanning tunneling microscopy, and density-functional theory-based supercell calculations. Comparing PdTe2 with its sister compound PtSe2, we demonstrate how enhanced interlayer hopping in the Te-based material drives a band inversion within the antibonding p-orbital manifold well above the Fermi level. We show how this mediates spin-polarized topological surface states which form rich multivalley Fermi surfaces with complex spin textures. Scanning tunneling spectroscopy reveals type-II superconductivity at the surface, and moreover shows no evidence for an unconventional component of its superconducting order parameter, despite the presence of topological surface states.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
PdTe2

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

1.7Pressure not reportedunknown
PdTe2

Archive — visibility unverified

Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

—Pressure not reportedunknown

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