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Detecting Superconductivity in the High Pressure Hydrides and Metallic Hydrogen from Optical Properties

J. P. Carbotte, E. J. Nicol, T. Timusk

DOI 10.1103/PhysRevLett.121.047002 · Physical Review Letters

T1

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Abstract

We present a new technique for measuring the critical temperature Tc in the high pressure, high Tc electron-phonon-driven superconducting hydrides. This technique does not require connecting leads to the sample. In the region of the absorption spectrum above the sum of the optical gap and maximum phonon energy, the reflectance mirrors the temperature variation of the superconducting order parameter. For an appropriately chosen value of fixed photon energy, the temperature dependence of the reflectance varies much more rapidly below T=Tc than above. It increases with increasing temperature in the superconducting state while it decreases in the normal state. Examining the temperature dependence of the reflectance at a fixed photon energy, there is a cusp at T=Tc which provides a measurement of the critical temperature. We discuss these issues within the context of the recently reported atomic metallic phase of hydrogen, but our proposed technique should prove useful for other hydrides with large coupling to high energy phonons.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
H3S

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

203155 GPaunknown
LaH10

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

260Pressure not reportedunknown
H3P

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

100Pressure not reportedunknown

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