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Extended Magnetic Dome Induced by Low Pressures in Superconducting FeSe1−xSx

S. Holenstein, J. Stahl, Z. Shermadini, G. Simutis, V. Grinenko, D. A. Chareev, R. Khasanov, J.-C. Orain, A. Amato, H.-H. Klauss, E. Morenzoni, D. Johrendt, H. Luetkens

DOI 10.1103/PhysRevLett.123.147001 · Physical Review Letters

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Abstract

We report muon spin rotation and magnetization measurements under pressure on Fe1+δSe1−xSx with x≈0.11. Above p≈0.6 GPa we find a microscopic coexistence of superconductivity with an extended dome of long range magnetic order that spans a pressure range between previously reported separated magnetic phases. The magnetism initially competes on an atomic scale with the coexisting superconductivity leading to a local maximum and minimum of the superconducting Tc(p). The maximum of Tc corresponds to the onset of magnetism while the minimum coincides with the pressure of strongest competition. A shift of the maximum of Tc(p) for a series of single crystals with x up to 0.14 roughly extrapolates to a putative magnetic and superconducting state at ambient pressure for x≥0.2.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
Fe1+δSe1-xSx

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8Pressure unresolvedunknown
FeSe

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8Pressure unresolvedunknown
FeSe

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377 GPaunknown
Fe1+δSe1-xSx

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—Pressure not reportedunknown
Fe1+δSe1-xSx

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—Pressure not reportedunknown
FeSe1-xSx

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

—Pressure not reportedunknown

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