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Unveiling Odd-Frequency Pairing around a Magnetic Impurity in a Superconductor

Vivien Perrin, Flávio L. N. Santos, Gerbold C. Ménard, Christophe Brun, Tristan Cren, Marcello Civelli, Pascal Simon

DOI 10.1103/PhysRevLett.125.117003 · Physical Review Letters

T1

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Abstract

We study the unconventional superconducting correlations caused by a single isolated magnetic impurity in a conventional s-wave superconductor. Because of the local breaking of time-reversal symmetry, the impurity induces unconventional superconductivity, which is even in both space and spin variables but odd under time inversion. We derive an exact proportionality relation between the even-frequency component of the local electron density of states and the imaginary part of the odd-frequency local pairing function. By applying this relation to scanning tunneling microscopy spectra taken on top of magnetic impurities immersed in a Pb/Si(111) monolayer, we show experimental evidence of the occurrence of the odd-frequency pairing in these systems and explicitly extract its superconducting function from the data.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
Pb

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1.8Pressure not reportedonset
Pb

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—Pressure not reportedunknown

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