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Reduction of the Spin Susceptibility in the Superconducting State of Sr2RuO4 Observed by Polarized Neutron Scattering

A. N. Petsch, M. Zhu, Mechthild Enderle, Z. Q. Mao, Y. Maeno, I. I. Mazin, S. M. Hayden

DOI 10.1103/PhysRevLett.125.217004 · Physical Review Letters

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Abstract

Recent observations [A. Pustogow et al., Nature (London) 574, 72 (2019).] of a drop of the O17 nuclear magnetic resonance (NMR) Knight shift in the superconducting state of Sr2RuO4 challenged the popular picture of a chiral odd-parity paired state in this compound. Here we use polarized neutron scattering (PNS) to show that there is a 34±6% drop in the magnetic susceptibility at the Ru site below the superconducting transition temperature. We measure at lower fields H∼13Hc2 than a previous PNS study allowing the suppression to be observed. The PNS measurements show a smaller susceptibility suppression than NMR measurements performed at similar field and temperature. Our results rule out the chiral odd-parity d=z^(kx±iky) state and are consistent with several recent proposals for the order parameter including even-parity B1g and odd-parity helical states.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
Sr2RuO4

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1.47Pressure not reportedunknown

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