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Magnetic Breakdown and Topology in the Kagome Superconductor CsV3Sb5 under High Magnetic Field

Ramakanta Chapai, Maxime Leroux, Vincent Oliviero, David Vignolles, Nicolas Bruyant, M. P. Smylie, D. Y. Chung, M. G. Kanatzidis, W.-K. Kwok, J. F. Mitchell, Ulrich Welp

DOI 10.1103/PhysRevLett.130.126401 · Physical Review Letters

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Abstract

The recently discovered layered kagome metals of composition AV3Sb5 (A=K, Rb, Cs) exhibit a complex interplay among superconductivity, charge density wave order, topologically nontrivial electronic band structure and geometrical frustration. Here, we probe the electronic band structure underlying these exotic correlated electronic states in CsV3Sb5 with quantum oscillation measurements in pulsed fields up to 86 T. The high-field data reveal a sequence of magnetic breakdown orbits that allows the construction of a model for the folded Fermi surface of CsV3Sb5. The dominant features are large triangular Fermi surface sheets that cover almost half the folded Brillouin zone. These sheets have not yet been detected in angle resolved photoemission spectroscopy and display pronounced nesting. The Berry phases of the electron orbits have been deduced from Landau level fan diagrams near the quantum limit without the need for extrapolations, thereby unambiguously establishing the nontrivial topological character of several electron bands in this kagome lattice superconductor.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
CsV3Sb5

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—Pressure not reportedunknown
KV3Sb5

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—Pressure not reportedunknown
RbV3Sb5

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

—Pressure not reportedunknown

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