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Diverse Manifestations of Electron-Phonon Coupling in a Kagome Superconductor

Jing-Yang You, Chih-En Hsu, Mauro Del Ben, Zhenglu Li

DOI 10.1103/PhysRevLett.134.106401 · Physical Review Letters

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Abstract

Recent angle-resolved photoemission spectroscopy (ARPES) experiments on the kagome metal CsV3Sb5 revealed distinct multimodal dispersion kinks and nodeless superconducting gaps across multiple electron bands. The prominent photoemission kinks suggest a definitive coupling between electrons and certain collective modes, yet the precise nature of this interaction and its connection to superconductivity remain to be established. Here, employing the state-of-the-art ab initio many-body perturbation theory computation, we present direct evidence that electron-phonon (e-ph) coupling induces the multimodal photoemission kinks in CsV3Sb5, and profoundly, drives the nodeless s-wave superconductivity, showcasing the diverse manifestations of the e-ph coupling. Our calculations well capture the experimentally measured kinks and their fine structures, and reveal that vibrations from different atomic species dictate the multimodal behavior. Results from anisotropic GW-Eliashberg equations predict a phonon-mediated superconductivity with nodeless s-wave gaps, in excellent agreement with various ARPES and scanning tunneling spectroscopy measurements. Despite the universal origin of the e-ph coupling, the contributions of several characteristic phonon vibrations vary in different phenomena, highlighting a versatile role of e-ph coupling in shaping the low-energy excitations of kagome metals.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
CsV3Sb5

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2.5Pressure unresolvedunknown
CsV3Sb5

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4.1Pressure not reportedunknown

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