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Anomalous Disappearance of High-Tc Superconductivity at High Hole Concentration in Metallic La2−xSrxCuO4

J. B. Torrance, Y. Tokura, A. I. Nazzal, A. Bezinge, T. C. Huang, S. S. P. Parkin

DOI 10.1103/PhysRevLett.61.1127 · Physical Review Letters

T1

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Abstract

Samples of La2−xSrxCuO4−δ have previously shown a maximum concentration of p=0.15 holes per [CuO2] unit, because increasing x>0.15 normally induces compensating oxygen vacancies. Annealing samples in 100 bars of oxygen pressure fills the oxygen vacancies and greatly increases the range of accessible hole concentrations, up to p=0.40 (or effectively Cu+2.40). We find that Tc is constant at ≃36 K from p=0.15 to 0.24, where it begins to decrease. Beyond p≃0.32, superconductivity disappears, even though the samples are more conducting.

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FormulaReported Tc (K)Pressure (GPa)Type
La2-xSrxCuO4-δ

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36Pressure not reportedonset

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