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Superconductivity of the Sr2Ca12Cu24O41 Spin-Ladder System: Are the Superconducting Pairing and the Spin-Gap Formation of the Same Origin?

Naoki Fujiwara, Nobuo Môri, Yoshiya Uwatoko, Takehiko Matsumoto, Naoki Motoyama, Shinichi Uchida

DOI 10.1103/PhysRevLett.90.137001 · Physical Review Letters

T1

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Abstract

Pressure-induced superconductivity in a spin-ladder cuprate Sr2Ca12Cu24O41 has not been studied on a microscopic level thus far although the superconductivity was already discovered in 1996. We have improved the high-pressure technique using a large high-quality crystal, and succeeded in studying the superconductivity using Cu63 nuclear magnetic resonance. We found that the anomalous metallic state reflecting the spin-ladder structure is realized and the superconductivity possesses an s-wave-like character in the meaning that a finite gap exists in the quasiparticle excitation: At a pressure of 3.5 GPa, we observed two excitation modes in the normal state from the relaxation rate T1−1. One gives rise to an activation-type component in T1−1, and the other T-linear component linking directly with the superconductivity. This gapless mode likely arises from free motion of holon-spinon bound states appearing by hole doping, and the pairing of them likely causes the superconductivity.

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FormulaReported Tc (K)Pressure (GPa)Type
Sr2Ca12Cu24O41

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2.83.5 GPaonset

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