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Effect of Irradiation-Induced Disorder on the Conductivity and Critical Temperature of the Organic Superconductor κ−(BEDT−TTF)2Cu(SCN)2

James G. Analytis, Arzhang Ardavan, Stephen J. Blundell, Robin L. Owen, Elspeth F. Garman, Chris Jeynes, Ben J. Powell

DOI 10.1103/PhysRevLett.96.177002 · Physical Review Letters

T1

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Abstract

We have introduced defects into clean samples of the organic superconductor κ−(BEDT−TTF)2Cu(SCN)2 in order to determine their effect on the temperature dependence of the interlayer conductivity σ and the critical temperature Tc. We find a violation of Matthiessen’s rule that can be explained by a model of σ involving a defect-assisted interlayer channel which acts in parallel with the bandlike conductivity. We observe an unusual dependence of Tc on residual resistivity, inconsistent with the generalized Abrikosov-Gor’kov theory for an order parameter with a single component, providing an important constraint on models of the superconductivity in this material.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
κ-(BEDT-TTF)2Cu(SCN)2

Archive — visibility unverified

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10Pressure not reportedonset
κ-(ET)2Cu[N(CN)2]Br

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

—Pressure not reportedunknown

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