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Evolution of interorbital superconductor to intraorbital spin-density wave in layered ruthenates

Austin W. Lindquist, Jonathan Clepkens, Hae-Young Kee

DOI 10.1103/PhysRevResearch.4.023109 · Physical Review Research

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Abstract

The ruthenate family of layered perovskites has been a topic of intense interest, with much work dedicated to the superconducting state of Sr2RuO4. Another long-standing puzzle is the lack of superconductivity in its sister compound, Sr3Ru2O7, which constrains the possible mechanisms of Sr2RuO4. Here we address a microscopic mechanism that unifies the orders in these materials. Beginning from a model of Sr2RuO4 featuring interorbital spin-triplet pairing via Hund's and spin-orbit couplings, we find that bilayer coupling alone enhances, while staggered rotations destroy interorbital superconductivity. A magnetic field then shifts van Hove singularities, allowing intraorbital spin-density wave order to form in Sr3Ru2O7. Our theory predicts that Sr3Ru2O7 without staggered rotations exhibits interorbital superconductivity with a possibly higher transition temperature.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
Sr2RuO4

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—Pressure not reportedunknown
Sr3Ru2O7

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

—Pressure not reportedunknown

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