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Higgs-Mediated Optical Amplification in a Nonequilibrium Superconductor

Michele Buzzi, Gregor Jotzu, Andrea Cavalleri, J. Ignacio Cirac, Eugene A. Demler, Bertrand I. Halperin, Mikhail D. Lukin, Tao Shi, Yao Wang, Daniel Podolsky

DOI 10.1103/PhysRevX.11.011055 · Physical Review X

T1

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Abstract

We propose a novel nonequilibrium phenomenon, through which a prompt quench from a metal to a transient superconducting state can induce large oscillations of the order parameter amplitude. We argue that this oscillating mode acts as a source of parametric amplification of the incident radiation. We report experimental results on optically driven K3C60 that are consistent with these predictions. The effect is found to disappear when the onset of the excitation becomes slower than the Higgs-mode period, consistent with the theory proposed here. These results open new possibilities for the use of collective modes in many-body systems to induce nonlinear optical effects.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
K3C60

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—Pressure not reportedunknown
Nb1-xTixN

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

—Pressure not reportedunknown
Bi2Sr2CaCu2O8+x

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—Pressure not reportedunknown
NbSe2

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—Pressure not reportedunknown

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