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Field-Induced Tuning of the Pairing State in a Superconductor

A. Rosuel, C. Marcenat, G. Knebel, T. Klein, A. Pourret, N. Marquardt, Q. Niu, S. Rousseau, A. Demuer, G. Seyfarth, G. Lapertot, D. Aoki, D. Braithwaite, J. Flouquet, J. P. Brison

DOI 10.1103/PhysRevX.13.011022 · Physical Review X

T1

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Abstract

The recently discovered superconductor UTe2, with a superconducting transition temperature Tc between 1.5 and 2 K, is attracting much attention due to strong suspicion of spin-triplet and topological superconductivity. Its properties under magnetic field are also remarkable, with field-reinforced (H∥b) and field-induced [H in the (b,c) plane] superconducting phases. Here, we report the first complete thermodynamic determination of the phase diagram for fields applied along the three crystallographic directions. For field along the easy a axis, we uncover a strong negative curvature of the upper critical field very close to Tc, revealing a strong suppression of the pairing strength at low magnetic fields. By contrast, measurements performed up to 36 T along the hard magnetization b axis confirm a bulk field-reinforced superconducting phase. Most of all, they also reveal the existence of a phase transition line within the superconducting phase. Drastic differences occur between the low-field and high-field phases pointing to different pairing mechanisms. Detailed analysis suggests a possible transition between a low-field spin-triplet to high-field spin-singlet state, a unique case among superconductors.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
UTe2

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1.45Pressure unresolvedonset
UTe2

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1.85Pressure unresolvedonset
UPt3

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—Pressure not reportedunknown
UGe2

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

—Pressure not reportedunknown
URhGe

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

—Pressure not reportedunknown
UCoGe

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

—Pressure not reportedunknown
URu2Si2

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

—Pressure not reportedunknown

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