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Robust and Clean Majorana Zero Mode in the Vortex Core of High-Temperature Superconductor (Li0.84Fe0.16)OHFeSe

Qin Liu, Chen Chen, Tong Zhang, Rui Peng, Ya-Jun Yan, Chen-Hao-Ping Wen, Xia Lou, Yu-Long Huang, Jin-Peng Tian, Xiao-Li Dong, Guang-Wei Wang, Wei-Cheng Bao, Qiang-Hua Wang, Zhi-Ping Yin, Zhong-Xian Zhao, Dong-Lai Feng

DOI 10.1103/PhysRevX.8.041056 · Physical Review X

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Abstract

The Majorana fermion, which is its own antiparticle and obeys non-Abelian statistics, plays a critical role in topological quantum computing. It can be realized as a bound state at zero energy, called a Majorana zero mode (MZM), in the vortex core of a topological superconductor, or at the ends of a nanowire when both superconductivity and strong spin orbital coupling are present. A MZM can be detected as a zero-bias conductance peak (ZBCP) in tunneling spectroscopy. However, in practice, clean and robust MZMs have not been realized in the vortices of a superconductor because of contamination from impurity states or other closely packed Caroli–de Gennes-Matricon (CdGM) states, which hampers further manipulations of MZMs. Here, using scanning tunneling spectroscopy, we show that a ZBCP well separated from the other discrete CdGM states exists ubiquitously in the cores of free vortices in the defect-free regions of (Li0.84Fe0.16)OHFeSe, which has a superconducting transition temperature of 42 K. Moreover, a Dirac-cone-type surface state is observed by angle-resolved photoemission spectroscopy, and its topological nature is confirmed by band calculations. The observed ZBCP can naturally be attributed to a MZM arising from the chiral topological surface state of a bulk superconductor. Thus, (Li0.84Fe0.16)OHFeSe provides an ideal platform for studying MZMs and topological quantum computing.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
(Li0.84Fe0.16)OHFeSe

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42Pressure not reportedunknown
(Li0.84Fe0.16)OHFeSe

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

42Pressure not reportedunknown
(Li0.75Fe0.25)OHFeSe

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—Pressure not reportedunknown

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