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Enhanced Coherent Terahertz Emission from Critical Superconducting Fluctuations in YBa2Cu3O6.6

D. Nicoletti, M. Rosenberg, M. Buzzi, M. Fechner, Y. Liu, S. Nakata, B. Keimer, R. A. Vitalone, D. N. Basov, P. E. Dolgirev, E. Demler, M. H. Michael, A. Cavalleri

DOI 10.1103/lbph-97sg · Physical Review X

T1

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Abstract

Coherent terahertz (THz) emission is emerging as a powerful new tool to probe symmetry breakings in quantum materials. This method relies on second order optical nonlinearities and is complementary to second harmonic generation spectroscopy. Here, we report coherent THz emission from Josephson plasmons in underdoped YBa2Cu3O6+x, and find that the amplitude of the emitted field increases dramatically close to the superconducting transition temperature, TC. We show theoretically how emission is enhanced by critical superconducting fluctuations, a nonlinear analog of critical opalescence. This observation is expected to be of general importance for the study of many thermal and quantum phase transitions.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
YBa2Cu3O6.6

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63Pressure not reportedunknown
YBa2Cu3O6.48

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51Pressure not reportedunknown
La1.905Ba0.095CuO4

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33Pressure not reportedunknown
YBa2Cu3O7-δ

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—Pressure not reportedunknown
Bi2Sr2CaCu2O8+δ

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—Pressure not reportedunknown
Tl2Ba2CaCu2O8+δ

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—Pressure not reportedunknown
La1.84Sr0.16CuO4

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—Pressure not reportedunknown
La1.885Ba0.115CuO4

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—Pressure not reportedunknown

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