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Observation of topological transition in high-Tc superconducting monolayer FeTe1−xSex films on SrTiO3(001)

X.-L. Peng, Y. Li, X.-X. Wu, H.-B. Deng, X. Shi, W.-H. Fan, M. Li, Y.-B. Huang, T. Qian, P. Richard, J.-P. Hu, S.-H. Pan, H.-Q. Mao, Y.-J. Sun, H. Ding

DOI 10.1103/PhysRevB.100.155134 · Physical Review B

T1

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Abstract

Superconductors with topological surface or edge states have been intensively explored for the prospect of realizing Majorana bound states, which obey non-Abelian statistics and are crucial for topological quantum computation. The traditional routes for making topological insulator/superconductor and semiconductor/superconductor heterostructures suffer fabrication difficulties and can only work at low temperature. Here, we use angle-resolved photoemission spectroscopy to directly observe the evolution of a topological transition of band structure nearby the Fermi level in two-dimensional high-Tc superconductor FeTe1−xSex/SrTiO3(001) monolayers, fully consistent with our theoretical calculations. Furthermore, evidence of edge states is revealed by scanning tunneling spectroscopy with assistance of theoretical calculations. Our study provides a simple and tunable platform for realizing and manipulating Majorana states at high temperature.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
FeTe1-xSex

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—Pressure not reportedunknown
FeTe1-xSex

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—Pressure not reportedunknown
FeSe

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65Pressure not reportedonset
FeTe0.55Se0.45

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—Pressure not reportedunknown
Bi2Pd

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—Pressure not reportedunknown

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