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de Haas–van Alphen effect investigation of the electronic structure of Al-substituted MgB2

A. Carrington, J. D. Fletcher, J. R. Cooper, O. J. Taylor, L. Balicas, N. D. Zhigadlo, S. M. Kazakov, J. Karpinski, J. P. H. Charmant, J. Kortus

DOI 10.1103/PhysRevB.72.060507 · Physical Review B

T1

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Abstract

We report a de Haas–van Alphen (dHvA) study of the electronic structure of Al-doped crystals of MgB2. We have measured crystals with ∼7.5% Al, which have a Tc of 33.6 K (∼14% lower than pure MgB2). dHvA frequencies for the σ-tube orbits in the doped samples are lower than in pure MgB2, implying a 16±2% reduction in the number of holes in this sheet of Fermi surface. The mass of the quasiparticles on the larger σ orbit is lighter than the pure case indicating a reduction in electron-phonon coupling constant λ. These observations are compared with band-structure calculations, and found to be in excellent agreement.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
Mg1-xAlx(B1-yCy)2

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—Pressure not reportedunknown
MgB2

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39Pressure not reportedunknown
MgB2

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38.5Pressure not reportedunknown
MgB2

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38.3Pressure not reportedonset
Mg0.921Al0.079B2

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33.6Pressure not reportedonset
Mg0.926Al0.074B2

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33.6Pressure not reportedonset
Mg0.921Al0.079B2

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34.4Pressure not reportedonset

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